† Corresponding author. E-mail:
Project supported by the National Key R&D Program of China (Grant No. 2016YFA0301603), the National Natural Science Foundation of China (Grant No. 11874341), Anhui Initiative in Quantum Information Technologies, and Chinese Academy of Sciences.
Quantum gas microscopy has enabled the study on intriguing properties of ultracold atoms in optical lattices. It provides the cutting-edge technology for manipulating quantum many-body systems. In such experiments, atoms have to be prepared into a two-dimensional (2D) system for being resolved by microscopes with limited depth of focus. Here we report an experiment on slicing a single layer of the atoms trapped in a few layers of pancake-shaped optical traps to create a 2D system. This technique is implemented with a microwave “knife”, i.e., a microwave field with a frequency defined by the resonant condition with the Zeeman-shifted atomic levels related to a gradient magnetic field. It is crucial to keep a stable preparation of the desired layer to create the 2D quantum gas for future experimental applications. To achieve this, the most important point is to provide a gradient magnetic field with low noises and slow drift in combination with a properly optimized microwave pulse. Monitoring the electric current source and the environmental magnetic field, we applied an actively stabilizing circuit and realized a field drift of 0.042(3) mG/hour. This guarantees creating the single layer of atoms with an efficiency of 99.92(3)% while atoms are hardly seen in other layers within 48 hours, satisfying future experimental demands on studying quantum many-body physics.
Ultracold atoms in optical lattices have been demonstrated to be very promising for studying quantum many-body physics.[1] In particular, quantum gas microscopy (QGM), composed of optical lattices and high-resolution imaging approaches, has becoming a cutting edge method for studying quantum crystals in a brand-new way.[2–7] Experiments such as measurement of Rényi entropy of a few-body system,[8] and in situ observation of many-body localization[9] have been performed with QGM, making it a unique tool for quantum simulation with ultracold atoms.
In three-dimensional (3D) lattices, it is of challenge to distinguish atoms in neighboring layers due to the fact that the depth of focus of the microscope is usually larger than the lattice constant. Moreover, the fluorescence emitted by out-of-focus atoms will blur the signal arising from the in-focus plane, damaging the imaging contrast. Therefore, it is important to prepare atoms in a monolayer for further studies. Furthermore, the 2D system is of great research interest for observing various quantum phenomena such as the Berezinsky–Kosterlitz–Thouless (BKT) transition.[10,11]
In principle, there are two different approaches to prepare 2D quantum gases. One is to compress a three-dimensional cloud of ultracold atoms with light sheets and load them into one layer of a one-dimensional (1D) optical lattices,[7,12] or into a surface trap.[13,14] The other approach, as demonstrated herein, starts with an 1D optical lattice consisting parallel pancake-like traps filled with atoms. Then a microwave “knife” is used to flip the internal state of one layer of the Zeeman-shifted atoms in the presence of a gradient magnetic field. The rest atoms which are not selected will be blown away from the system by a resonant laser beam.[3,4,15,16,6]
In order to perform future experiments with a prepared 2D system, repeatedly producing the 2D system with high stability is of key importance. This would ensure the high-fidelity manipulation of many-body quantum state and a sufficient signal-to-noise ratio (SNR) during imaging. A low fluctuation of the number of atoms favors the evaporative cooling to achieve lower temperatures for studying quantum phenomena. For example, a low temperature is critical to create unity filling Mott insulators[17,18] and to observe antiferromagnetic correlations[19,20] in optical lattices.
With this approach, the major challenges for preparing a 2D quantum gas are: Firstly, to provide a gradient magnetic field with low noises and slow drifts; Secondly, to compose a microwave pulse for coupling relevant atomic levels with high fidelity. Here we report on the techniques we developed to meet these demands. Briefly, based on the measured signal with a Hall sensor the current noise of the power supply is suppressed by a fast feedback circuit and the current drift is corrected. The environmental magnetic field is monitored by a fluxgate type sensor and its drift is further compensated with a pair of Helmholtz coils whose current is delivered by an ultra-stable power supply. A microwave Landau–Zener transfer process is used to flip the internal state of atoms. The achieved efficiency, 99.92(3)%, of flipping atomic states indicates the performance of noise suppression. A repeated measurement on the spatial drift of the flipped atoms calibrates the drift of the magnetic field as 0.042(3) mG/hour, which outperforms the best results reported in a couple similar experiments.[16,21] In the following, we describe the experimental setup in Section
Our experimental setup is shown in Fig.
Beneath the chamber, a high-resolution objective situates with a numerical aperture of 0.8. The imaging resolution was calibrated to be 690 nm for the emitted light with a wavelength of 780 nm (87Rb DII line). Meanwhile, the inner surface of the this viewport is coated with a high-reflective (HR) coating for the wavelength of 1064 nm. The incident laser beam of 1064 nm and its reflected beam from the inner surface together form the Z-lattice whose period is 532 nm. The X and Y lattices are both built by a pair of 532 nm laser beams crossed at the center with an angle of 50° resulting in a lattice constant of 630 nm. During fluorescence imaging, all the three lattices are raised to the maximal depth to pin the atoms on their own lattice sites.
After the BEC is achieved, the laser intensity of the Z-lattice is ramped up gradually and the atoms are loaded into a few layers of this lattice. Monolayer selection is performed with a Landau–Zener crossing (LZC) process,[22] which is implemented by a microwave knife. The gradient magnetic field is generated by two pairs of coils mounted outside the chamber. The microwave field is delivered by an antenna placed on top of the upper viewport for approaching the atoms as close as possible.
A single-axis fluxgate (FL-200, StefanMayer Instrument) with a bandwidth of 1 kHz and a range of ± 2 G is placed about 3 cm away from the atoms to monitor the magnetic field along the Z direction. By adding three pairs of Helmholtz coils surrounding the chamber, we can generate bias fields along each direction to compensate for the stray magnetic field and adjust the direction of magnetic field gradient. The process will be described in detail in the following sections.
As mentioned above, the BEC atoms are loaded into a few layers of the Z-lattice by ramping up its trapping depth to kB × 3.2 μ K corresponding to an axial trapping frequency of 2π × 24 kHz. We use two states in the ground state 52S1/2 for the monolayer selection, i.e. |F = 1,mF = −1⟩ and |F = 2, mF = −2⟩, labeled by |↓⟩ and |↑⟩, respectively. Therefore, we also refer to the process of transferring between |↓⟩ and |↑⟩ as “spin flip”. The gradient magnetic field is applied along the Z direction. Therefore, the Zeeman energy splitting of the atoms becomes spatially dependent.
To select one layer of the atoms in the Z-lattice, we take the following steps sequentially. First, all the atoms originally prepared in |↓⟩ are transferred to |↑⟩ with a global microwave sweep, an LZC pulse explained later in Section
To perform spin flip for the atoms in one particular layer while leaving the rest unchanged, it is necessary to create spatially dependent energy splitting along the Z axis with a gradient magnetic field. Two points should be considered carefully. One is that the magnetic field gradient should be strong enough to make the energy splitting of atoms in neighboring layers highly distinguished by the second microwave pulse. The other one is that the magnetic field in the target layer should be homogeneous for a high-fidelity spin-flip of all the atoms. Write the gradient as
In total, we generate a magnetic field gradient of 100 G/cm combined with an offset magnetic field of 35 G at Z direction. Ideally, atoms should be prepared close to the center of the gradient coils at which gradient coils create zero magnetic field, so that the current noise of power supply can only bring little magnetic noise to atoms. However, the focus of the high-resolution objective, where the target layer should be located, was aligned 1 mm below the gradient center due to assembly deviation. Then, the total field strength at the position of the target layer is |Btotal| = 0.1 cm × 100 G/cm + 35 G = 45 G, proportional to the current of the power supplies. Thus, the atoms suffer directly from the current noises arising from the relevant power supplies.
The radius of the atom cloud in our experiment is smaller than 50 μm. In this region, we realize a very flat magnetic field in the X–Y plane as |Btotal(50 μm)| − |Btotal(0)| < 0.7 mG. Meanwhile, the lattice constant in the Z direction, 532 nm, results in a Δ B = 5.32 mG (equivalent to a Zeeman shift of 2.1 × 5.32 = 11.17 kHz) difference between the neighboring layers. Therefore, equation (
As the strong magnetic fields require large electric currents which cause dramatically heating to the coils, water cooling is employed to stabilize the temperature of these coils. Suppressing the temperature fluctuation of the coils is of great importance for two aspects: Firstly, the thermal deformation of the coils is reduced, which results in a precisely stable magnetic field around the target layer of atoms. Secondly, the thermal disturbance to the surrounding air is reduced, which results in a stable refractive index favorable for stabilizing the beam paths. Here the coils are made of hollow copper wires with the central hole radius of 1.25 mm for injecting temperature actuated water. Meanwhile, the temperatures of the coils are monitored by sensors (Texas Instruments, LM35DZ) as reference to prevent overheating.
Transferring 87Rb atoms between |↓⟩ and |↑⟩ can be performed either by Rabi π pulses[23] or the adiabatic LZC.[22] However, the former is more sensitive to magnetic noises since the phase and amplitude of Rabi oscillations could be modified by the magnetic fluctuations by changing the detunings. In contrast, the latter has a much higher tolerance to magnetic noises. Therefore, we employ the LZC in our experiment for flipping the atomic sates.
The Zeeman splitting of |↑⟩ and |↓⟩ is 2.1 kHz/mG and the magnetic field gradient induces an energy difference of 11.17 kHz between neighboring layers. Thus, we perform a microwave LZC by sweeping its frequency from −4 kHz to 4 kHz with respect to the resonant frequency.
The time dependence of the microwave frequency and strength is of key importance for the transfer efficiency. To achieve a high efficiency, we use a hyperbolic secant (HS1) pulse[24] whose Rabi frequency Ω(t) and frequency detuning Δ(t) are defined as follows:
Figure
In our experiment, we measured the transfer efficiency when applying the HS1 pulse to a cloud of BEC atoms in a homogeneous magnetic field of 1 G along the Z direction. All the atoms N0 in |↓⟩ are first transferred to |↑⟩ by a microwave LZC pulse and subsequently back to |↓⟩ by a second identical pulse. Then the number of atoms in |↑⟩ is measured as N|↑⟩. With the knowledge of N0 and N|↑⟩, we can derive the transfer efficiency η given the following relations
To determine the sign in the expression of η±, we measure the number of spin-up atoms after applying the first LZC pulse. When the measured number is larger than N0/2, we choose +. Otherwise, we choose −. Shown in Fig.
The Rabi frequency of the pulse is proportional to the square root of the microwave power. Measuring the Rabi oscillation of the atoms under a microwave power of 2 dBm delivered by the signal generator, we calibrate the Rabi frequency as 3.21(2) kHz. Under the magnetic field with a gradient of 100 G/cm, we set a sweep range of ± 800 kHz, a pulse length of 20 ms, and a Rabi frequency of 14 kHz to flip the atoms in all layers. This is called a global flip. In contrast, a range of ± 4 kHz, a pulse length of 4 ms and a Rabi frequency of 3.21 kHz are employed to flip a single layer of interest. This is called a single flip. Its efficiency is measured to be 99.92(3)%.
In principle, a shorter HS1 pulse with a higher Rabi frequency and a reduced sweep range could also be used without decreasing the efficiency under the condition of on resonance. However, with such a pulse, the two edges of the efficiency curve in Fig.
In our experiment, a typical spin-flip efficiency reaches over 99%. However, there are still about hundred atoms remained in their initial state |↓⟩ after a global flip over more than 105 atoms. These atoms will create noises during final detection by fluorescence imaging. Hence, we use a σ− polarized repump laser resonant with |↓⟩ → |52 P3/2, F = 2⟩ to transfer them to |↑⟩ via a spontaneous Raman transition |↓⟩ → |52 P3/2, F = 2 ⟩ → |↑⟩.
After the single flip pulse, only atoms in the target layer are transferred back to |↓⟩, while the rest in other layers still remain in |↑⟩. They are removed with a σ− laser, the push-out laser, resonant with the circling transition |↑⟩ ← |52 P3/2, F = 3⟩. Therefore, no dark state involves in this process resulting in a removal efficiency >99%.
Intuitively, the single-layer selection requires the noise and drift of the magnetic field to be much lower than ΔB. A numerical simulation on the LZC process shows that the magnetic fluctuation should be lower than 1 mG for maintaining a spin-flip efficiency over 99%. Since the magnetic field around the atoms is about 45 G, this corresponds to a noise level of 22 ppm. In principle, it is straightforward to detect the magnetic field with a sensor and then stabilize the field strength to a certain value by an active feedback circuit.[25–27] In our experiment, however, the magnetic field is too strong (∼ 45 G) that no available sensor provides a proper precision at such a strength. To satisfy this stringent request, we employ three approaches: (a) Suppress the electronic noise of the current supply with a fast feedback circuit. (b) Compensate for the drift of the magnetic field induced by the drift of current supply. (c) Compensate for the drift of environmental magnetic field.
The offset coils and the gradient coils create magnetic fields at the position of atoms with the factors of 1.75 G/A and 0.1 G/A, respectively (see Fig.
We designed a noise reduction system with an insulated-gate bipolar transistor (IGBT) and a Hall sensor (LEM, ITN 600-S). The power supply, gradient coils and the IGBT are connected in series. The Hall sensor detects the current in coils and delivers a scaled current. This signal is then transformed into a voltage with a sampling resistor which has an extremely low temperature coefficient of 0.5 ppm/K. Afterwards, this voltage is fed into a PID electronic board which provides the driving signal for the gate of IGBT.
The rms noise is suppressed to 0.6 mA at the working current of 100 A as shown in Fig.
The long-term drift of current is destructive for the repeatability of selecting the same single layer of atoms. Though the above noise reduction circuit has a bandwidth covering low frequencies, we still observe an obvious drift of the current running in either the offset coils or the gradient coils per other Hall sensors (LEM, ITN 600-S). Based on the measured value of current in the offset coils, the induced drift of the magnetic field is actively compensated by a pair of Helmholtz coils (C1) made of one winding of wire. The C1 coils generate a bias field with the factor of 50 mG/A and are powered by an analog-controlled current supply (HighFinesse BCS 2 A/25 V). One easily finds that a current of 35 mA in C1 compensates the drift of magnetic field induced by the current drift of 1 mA in the offset coils. This scheme offers a fine compensation. Therefore, it is used as well for compensating the drift of current in the gradient coils.
The noise and drift of the current in the magnetic coils are suppressed with the above two approaches. Finally, the drift of the environmental magnetic field should be considered.
Measuring the Rabi oscillation between two hyperfine levels of the atoms shows that the noise of the environmental magnetic field along the Z direction is around 0.4 mG, which agrees with the measurement by a fluxgate-type sensor. Therefore the noise of the environmental magnetic field has a negligible impact on the efficiency of single-layer selection. However, the slow drift of the environmental magnetic field is on the level of a few mG and has a larger impact. Thus, we implement a static compensation approach. Before each experimental trial, we turn off the currents in all coils and measure the background magnetic field for 1 s with a fluxgate sensor. The measured value is acquired by a computer, then an appropriate current will be calculated and fed into the compensation coil of C1 with the help of the real-time control system. This process is carried out automatically in every experimental trail.
Based on the above three approaches, both the noise and drift of the magnetic field around the atoms are suppressed. The performance of the whole solution is characterized by directly testing the response of the atoms.
Ideally, the magnetic field gradient should be well aligned along the Z direction and orthogonal to the plane of each layers. However, in the experiment, the tilt of the coils as well as a background magnetic field may change the direction of the magnetic field gradient, resulting in a misalignment. Suppose a background magnetic field along the X direction (B = Bex), an angle θ will be created between the direction of gradient and the Z axis as
As shown in Fig.
In order to study the drift of magnetic field around the atoms, we run the above experiment repeatedly to monitor the drift of fringes. An 8-hour measurement was performed, as shown in Fig.
Besides the three approaches introduced in Section
It is worth mentioning that some groups synchronize their experimental sequence to the AC line phase to reduce the influence of 50 Hz noise.[21,28] However, according to our test, it is unnecessary to do so since the above approaches suppress such a noise effectively. After the misalignment of magnetic field gradient is corrected, we always achieve an efficiency higher than 99% for preparing the single layer which does not depend on the synchronization. Figure
We have developed a technique on preparing a 2D quantum gas based on slicing a single layer of atoms trapped in a few layers of pancake-shaped optical traps. To achieve a high efficiency for this preparation, a Landau–Zener-cross microwave pulse with well-designed profile is applied to improve the noise tolerance and stability. The rms noise of magnetic field induced by the current supplies is reduced to 0.36 mG with a home-built noise reduction system. The slow drift of magnetic field is minimized with a static compensation circuit and a more stable water chiller. The effectiveness of these approaches was verified by observing the response of atoms with in situ microscopic imaging. Finally a slow drift speed of 0.042(3) mG/hour is achieved, promising a continuous experiment of 48 hours for maintaining the preparation efficiency of the 2D quantum gas as 99.92(3)%. Synchronizing the experimental sequence to the phase of the AC line is found to be unnecessary for achieving the high efficiency.
Our work can be extended to the creation of a bilayer lattice system, in which disentangling two layers to create a low-entropy single layer system is proposed.[29] Meanwhile, the home-made ultrastable current supply and the full scheme of stabilizing magnetic fields have promising applications in both scientific researches and various industries.
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